In this paper, from the standpoint of Raman spectrum research aspect in material science, Raman spectrum analysis of graphite and diamond microcrystal retained by gallium phosphide nanoparticles is introduced. We found that molecular configuration of basic fuchsin adsorbed on gallium phosphide nanoparticles through experiments. Based on these, Raman scattering is used for analyzing basic fuchsin adsorbed on surface of gallium phosphide nanoparticles. Moreover, we discuss the corresponding meanings of agglomeration phenomenon from the perspective of material.